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Magnetic anisotropy and superspin glass behaviour of Fe nanoparticles embedded in Cr and Ag matrices

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journal contribution
posted on 21.10.2015, 10:04 by D. Peddis, M. T. Qureshi, Stephen H. Baker, Chris Binns, Mervyn Roy, S. Laureti, D. Fiorani, P. Nordblad, R. Mathieu
Static and dynamical magnetic properties of Fe nanoparticles (NPs) embedded in non - magnetic (Ag) and antiferromagnetic (Cr) matrices with a volume filling fraction (VFF) of 10% have been investigated . In both Fe@Ag and Fe@Cr nanocomposites , the Fe nanoparticles have a narrow size distribution, with a mean particle diameter around 2 nm. In both samples , the saturation magnetization reaches that of Fe bulk bcc, suggesting the absence of alloying with the matrices. The coercivity at 5 K is much larger in Fe@Cr than in Fe@Ag as a result of the strong interaction between the Fe NPs and the Cr matrix. Temperature - dependent magnetization and ac - susceptibility measurements point out further evidence of the enhanced inter - particle interaction in the Fe@Cr system . While the behavior of Fe@Ag indicates the presence of weakly interacting magnetic monodomain particles with a wide distribution of blocking temperatures , Fe@Cr behaves like a superspin glass produced by the magnetic interaction between nanoparticles.

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Citation

Philosophical Magazine, 2015, doi: 10.1080/14786435.2015.1090640

Author affiliation

/Organisation/COLLEGE OF SCIENCE AND ENGINEERING/Department of Physics and Astronomy

Version

AM (Accepted Manuscript)

Published in

Philosophical Magazine

Publisher

Taylor & Francis (Routledge)

issn

0950-0839

eissn

1362-3036

Acceptance date

29/08/2015

Copyright date

2015

Available date

27/10/2016

Publisher version

http://www.tandfonline.com/doi/abs/10.1080/14786435.2015.1090640

Notes

The file associated with this record is under a 12-month embargo from publication in accordance with the publisher's self-archiving policy, available at http://authorservices.taylorandfrancis.com/sharing-your-work/. The full text may be available in the publisher links provided above.

Language

en

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